流延成型技术制备片状氮化硅陶瓷研究进展

doi:10.3969/j.issn.1001-1935.2025.02.016

耐火材料 ›› 2025, Vol. 59 ›› Issue (2): 177-184.DOI: 10.3969/j.issn.1001-1935.2025.02.016

• 综合评述 • 上一篇

流延成型技术制备片状氮化硅陶瓷研究进展

赵辰啸, 李世鹏, 王刚, 周玉栋, 袁波

中钢集团洛阳耐火材料研究院有限公司先进耐火材料全国重点实验室河南洛阳 471039

收稿日期:2024-08-07 出版日期:2025-04-15 发布日期:2025-04-14
通讯作者: 袁波,男,1983年生,博士,高级工程师。E-mail:boyuan0401@163.com
作者简介:赵辰啸:男,2000年生,硕士研究生。E-mail:15530090311@163.com

Research progress on preparation of sheet-like silicon nitride ceramics by tape-casting technology

Zhao Chenxiao, Li Shipeng, Wang Gang, Zhou Yudong, Yuan Bo

First author’s address:State Key Laboratory of Advanced Refractories,Sinosteel Luoyang Institute of Refractories Research Co.,Ltd.,Luoyang 471039,Henan,China

Received:2024-08-07 Online:2025-04-15 Published:2025-04-14

摘要/Abstract

摘要： 综述了国内外关于流延成型技术制备氮化硅陶瓷的原理和流程,阐述了有机和水基流延浆料体系中各种添加剂的特点和工艺流程参数对流延效果的影响,总结了流延成型技术制备片状氮化硅陶瓷的研究进展及仍存在的问题,同时探讨该技术未来的发展方向。

关键词: 氮化硅陶瓷, 流延成型, 有机流延体系, 水基流延体系

Abstract: The principles and processes of preparing silicon nitride ceramics by tape-casting technology in China and aboard were reviewed.The characteristics of various additives in both organic and water-based tape-casting slurry systems as well as the influence of process parameters on the tape-casting effect were elaborated.The research progress and existing problems in the preparation of sheet-like silicon nitride ceramics by tape-casting technology were summarized.The future development direction of this technology was discussed.

Key words: silicon nitride ceramics, tape-casting, organic tape-casting system, water-based tape-casting system

中图分类号:

TQ175

赵辰啸, 李世鹏, 王刚, 周玉栋, 袁波. 流延成型技术制备片状氮化硅陶瓷研究进展[J]. 耐火材料, 2025, 59(2): 177-184.

Zhao Chenxiao, Li Shipeng, Wang Gang, Zhou Yudong, Yuan Bo. Research progress on preparation of sheet-like silicon nitride ceramics by tape-casting technology[J]. Refractories, 2025, 59(2): 177-184.

参考文献

[1] 董其政.环保非水基流延成型制备高质量氧化锆陶瓷基片及氮化硅生坯的研究[D].景德镇:景德镇陶瓷大学,2018.
[2] 曹飞.陶瓷大板成型工艺及其装备应用分析[J].佛山陶瓷,2020,30(9):31-36.
[3] 王月隆.氮化硅粉体合成及其高导热陶瓷的组织与性能研究[D].北京:北京科技大学,2022.
[4] JABBARI M,BULATOVA R,TOK A I Y,et al.Ceramic tape casting:A review of current methods and trends with emphasis on rheological behaviour and flow analysis[J].Materials Science and Engineering:B,2016,212:39-61.
[5] 李淑静,李楠.陶瓷胶态成型方法研究新进展[J].耐火材料,2005,39(2):135-139.
[6] HOWATT G N,BRECKENRIDGE R G,BROWNLOW J M.Fabrication of thin ceramic sheets for capacitors[J].Journal of the American Ceramic Society,1947,30(8):237-242.
[7] OTSUKA K,OHSAWA Y,YAMADA K.A study on the alumina ceramics casting conditions by the doctor-blade method and their effect on the properties of green tape (part 1)[J].Journal of the Ceramic Association,Japan,1986,94(1087):351-359.
[8] CHOU Y T,KO Y T,YAN M F.Fluid flow model for ceramic tape casting[J].Journal of the American Ceramic Society,1987,70(10):C-280-C-282.
[9] 李冬云,乔冠军,金志浩.流延法制备陶瓷薄片的研究进展[J].硅酸盐通报,2004,23(2):44-47.
[10] 谢雨洲,彭超群,王小锋,等.流延成型技术的研究进展[J].中国有色金属学报,2015,25(7):1846-1857.
[11] TADROS T F.Rheology of dispersions:Principles and applications[M].Weinheim:Wiley-VCH,2010.
[12] ZENG Y P,KONDO N,HIRAO K,et al.The anisotropic properties of the tape cast Si₃N₄ ceramics with rod-like β-Si₃N₄ seeds addition[J].Key Engineering Materials,2006,317/318:593-596.
[13] 张景贤,段于森,江东亮,等.高导热Si₃N₄陶瓷基片材料的制备研究[J].真空电子技术,2016(5):7-10.
[14] 文科林,栾道成,左城铭,等.烧结助剂及增强相对氮化硅陶瓷材料性能的影响[J].中国陶瓷,2021,57(8):26-32.
[15] 周泊岸,唐志红,李哲,等.氮化硅陶瓷低温烧结助剂研究进展[J].化工矿物与加工,2024,53(1):69-75.
[16] 周玉栋,李世鹏,王文武,等.高导热氮化硅陶瓷的制备研究进展[J].耐火材料,2024,58(3):270-276.
[17] 欧阳雪琼,黎达,孙国立,等.陶瓷材料流延成型工艺的研究进展[J].佛山陶瓷,2023,33(2):1-4+31.
[18] 宋占永,董桂霞,杨志民,等.陶瓷薄片的流延成型工艺概述[J].材料导报,2009,23(9):43-46.
[19] 吕子彬,海韵,吕金玉,等.陶瓷基片流延成型用浆料研究进展[J].武汉理工大学学报,2021,43(6):7-14.
[20] 赵兴祥.球磨法对Si₃N₄粉体表面改性及其在水中分散性能的研究[D].烟台:烟台大学,2019.
[21] LIU Y,CHENG L J,LI H,et al.Formation mechanism of stereolithography of Si₃N₄ slurry using silane coupling agent as modifier and dispersant[J].Ceramics International,2020,46(10):14583-14590.
[22] 陈殿营,张宝林,庄汉锐,等.氮化硅流延膜的制备[J].硅酸盐通报,2003,22(6):71-74.
[23] 王铃沣,周泊岸,段于森,等.氮化硅陶瓷基板制备及其金属化研究[J].化工矿物与加工,2024,53(2):12-19.
[24] HOU Q D,LUO X D,XIE Z P,et al.Development of the environmental friendly non-aqueous tape casting process for high-quality Si₃N₄ ceramic substrates[J].IOP Conference Series:Materials Science and Engineering,2019,678(1):012042.
[25] BITTERLICH B,HEINRICH J G.Aqueous tape casting of silicon nitride[J].Journal of the European Ceramic Society,2002,22(13):2427-2434.
[26] LIU S C,YE F,LIU L M,et al.Feasibility of preparing of silicon nitride ceramics components by aqueous tape casting in combination with laminated object manufacturing[J].Materials & Design (1980-2015),2015,66:331-335.
[27] KULIG M,GREIL P.Surface chemistry and suspension stability of oxide-nitride powder mixtures[J].Journal of Materials Science,1991,26(1):216-224.
[28] 郗威,周杨杨,刘鹏飞,等.球磨介质对氮化硅粉体的微观形貌和表面氧化硅层的影响[J].中国粉体技术,2023,29(6):82-90.
[29] REN L C,LUO X F,ZHOU H Q.The tape casting process for manufacturing low-temperature co-fired ceramic green sheets:A review[J].Journal of the American Ceramic Society,2018,101(9):3874-3889.
[30] REN L C,LUO X F,XIA Y S,et al.Fabrication of a high-performance film based borosilicate glass/Al₂O₃ ceramics for LTCC application[J].Journal of the European Ceramic Society,2017,37(6):2415-2421.
[31] 李鹏飞,吴长友,周靖仁,等.陶瓷用聚合物分散剂的制备及应用研究进展[J].中国陶瓷,2012,48(11):4-10+18.
[32] ZHAO H,TANG F,XIE Y Z,et al.Fabrication and rheological behavior of tape-casting slurry for ultra-thin multilayer transparent ceramics[J].International Journal of Applied Ceramic Technology,2020,17(3):1255-1263.
[33] 赵芃,谢光远,宗红军,等.氧化锆PVA-水基流延成型工艺研究[J].硅酸盐通报,2016,35(10):3336-3339.
[34] ZHANG J X,YE F,JIANG D L,et al.Preparation of bulk Si₃N₄ from tape casting and lamination[J].Ceramics International,2006,32(3):277-282.
[35] 黄智勇,王翔,刘学建,等.氮化硅粉体的行星式球磨工艺研究[J].陶瓷科学与艺术,2003,37(6):21-25.
[36] 葛成灿,王源升,余红伟,等.泡沫及消泡剂的研究进展[J].材料开发与应用,2010,25(6):81-85.
[37] 崔唐茵,刘镇,魏春城.流延成型技术制备陶瓷薄片的研究现状[J].中国陶瓷工业,2022,29(5):39-44.
[38] 王伟伟.层状Si₃N₄基陶瓷材料的制备与性能研究[D].淄博:山东理工大学,2020.
[39] 刘镇.高韧性层状氮化硅陶瓷材料的制备及性能研究[D].淄博:山东理工大学,2021.
[40] 叶枫,刘仕超,高晔,等.一种水基流延成型制备致密氮化硅陶瓷材料及致密异形氮化硅陶瓷材料的方法:CN103922746B[P].2015-07-22.
[41] 向军辉,黄勇.薄片陶瓷材料凝胶流延成型(Gel-Tape-Casting)工艺研究[J].材料导报,2000(Z10):105-107.
[42] 付杰,刘源,赵振威,等.Y₂O₃-MgO外加量对Isobam凝胶流延氮化硅性能的影响[J].耐火材料,2024,58(5):400-404.
[43] CHARTIER T,PENARROYA R,PAGNOUX C,et al.Tape casting using UV curable binders[J].Journal of the European Ceramic Society,1997,17(6):765-771.

流延成型技术制备片状氮化硅陶瓷研究进展

Research progress on preparation of sheet-like silicon nitride ceramics by tape-casting technology

PDF

可视化

摘要/Abstract

引用本文

使用本文

参考文献

相关文章 4

编辑推荐

Metrics

本文评价

[1]	付杰, 刘源, 赵振威, 孔源, 杨露君, 王安修, 马成良. Y₂O₃-MgO外加量对Isobam凝胶流延氮化硅性能的影响[J]. 耐火材料, 2024, 58(5): 400-404.
[2]	周玉栋, 李世鹏, 王文武, 张一帆, 赵辰啸. 高导热氮化硅陶瓷的制备研究进展[J]. 耐火材料, 2024, 58(3): 270-276.
[3]	余冬玲, 张会玲, 罗宏斌, 冯晓宇, 吴南星. MgO和Y₂O₃对气压烧结制备氮化硅陶瓷的影响[J]. 耐火材料, 2021, 55(4): 316-318.
[4]	孙钦英，朱秀英 . 发动机用新材料──氮化硅陶瓷 [J]. , 1994, 28(2): 108-112.